The most useful (but the hardest) method; having a ULTIMATE PKMN-CATCHING TEAM;
~ Train a Dusclops w/ Spite, Protect, Subsitute and Torment.
~ Train a Umbreon w/ Mean Look, BPass, Screech and Charm.
~ Train a Scizor w/ BPass, False Swipe, Sonicboom and Light Screen.
~ Train a Wobbuffet w/ Encore, Counter, Magic Coat and Safeguard.
~ Train a Crobat w/ Mean Look, Taunt, Protect and Sunny Day.
~ Train a Mawile w/ Sweet Scent, Sing, BPass and Fake Tears.
Have your Umbreon at the lead. Use Mean Look when you see him and use Screech and Charm 'till you can't use them anymore, than BPass to Scizor. With Scizor, use Light Screen first, Sonicboom a few times and FSwipe until his/her HP becomes 1; then BPass to Mawile. With Mawile, put him to sleep and use Fake Tears and SScent until you can't use them anymore. Then, BPass to Dusclops and use Torment-Protect combo. Use Spite if he manages to hit you, and start chucking Ultra/Timer Balls to him. Wobbuffet and Crobat are back-ups in case he kills any of you PKMN. To avoid this, train these PKMN to Lv50 or higher.
NOTE: Finding LegenDogz is way hard. There are NO tricks to make them appear on any route, that part is PURE LUCK. The team I prefer is for catching em easily when you see him/her, especially if you don't want to waste your Master on him.
EDIT: I caught my Latias on Sapphire, Latios on Ruby, Suicune on FireRed, and Entei on LeafGreen with this method. I was lucky, as it took me 30 mins to find both
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